Advanced Energy Materials
01 December 2020
Beyond d Orbits: Steering the Selectivity of Electrochemical CO2 Reduction via Hybridized sp Band of Sulfur‐Incorporated Porous Cd Architectures with Dual Collaborative Sites
Yunzhen Wu1, Panlong Zhai1, Shuyan Cao1, Zhuwei Li1, Bo Zhang1, Yanting Zhang1, Xiaowa Nie1, Licheng Sun1,2,3, and Jungang Hou1
1 State Key Laboratory of Fine Chemicals, School of Chemical Engineering, Dalian University of Technology (DUT), Dalian, 116024 P. R. China
2 Center of Artificial Photosynthesis for Solar Fuels, School of Science, Westlake University, Hangzhou, 310024 P. R. China
3 Department of Chemistry, School of Engineering Sciences in Chemistry, Biotechnology and Health, KTH Royal Institute of Technology, Stockholm, 10044 Sweden
10.1002/aenm.202070183
In article number 2002499, Jungang Hou and co-workers report a sulfur-incorporated porous Cd architecture with superior activity for selective CO generation. The linear scaling relations are naturally eliminated, enabling the convenient modulation of selectivity for CO2 reduction toward CO rather than HCOOH. The covalently hybridized sp band system with dual collaborative sites is vividly visualized by the inseparable king bird in this picture.
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